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Photophysics and Photochemistry of a BODIPY‐Based Photosensitizer by Karl Michael Ziems
Photophysics and Photochemistry of a BODIPY‐Based Photosensitizer by Karl Michael Ziems
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Photophysics and Photochemistry of a BODIPY‐Based Photosensitizer

Quantumchemical Simulations
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Description

Karl Michael Ziems investigates a meso-mesityl-2,6-Iodine substituted Boron Dipyrromethene (BODIPY) dye regarding its functionality as photosensitizer in a two-component light-driven hydrogen evolution. The author uses quantum chemical calculations performed at the time-dependent density functional (TDDFT) and multi-state restricted active space perturbation theory through second-order (MS-RASPT2) level of theory. The light-induced processes associated with the formation of the active photosensitizer, i.e., by means of charge separation, as well as the population of undesired degradative pathways are elucidated. Hereby, the two proposed and investigated mechanisms are based on a heavy atom effect of iodine in the (excited) singlet/triplet manifold and preliminary reduction (of the dye) by a sacrificial electron donor and subsequent photoexcitation.

Author Biography:

Karl Michael Ziems obtained his Master of Science in chemistry at the Friedrich Schiller University Jena, and conducted his Master’s thesis in the field of quantum chemistry. Currently, he studies theoretical and computational chemistry at the University of Oxford.
Release date Australia
May 6th, 2019
Audience
  • Professional & Vocational
Edition
1st ed. 2019
Illustrations
1 Illustrations, black and white; XIII, 139 p. 1 illus.
Pages
139
ISBN-13
9783658261870
Product ID
30295160

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